New alpha-substituted succinate-based hydroxamic acids as TNFalpha convertase inhibitors

J Med Chem. 1999 Nov 18;42(23):4890-908. doi: 10.1021/jm990377j.

Abstract

Tumor necrosis factor alpha convertase (TACE), the enzyme responsible for the processing of pro-TNFalpha to TNFalpha, has been reported to be a metalloproteinase closely related to matrix metalloproteinases (MMPs). Current inhibitors of TACE such as succinate-based hydroxamic acids exemplified by Marimastat (TACE IC(50): 3.8 nM; blood IC(50): 7 microM) and BB1101 (TACE IC(50): 0.2 nM; blood IC(50): 2.3 microM) suffer from modest potency in blood and poor in vivo properties. The introduction of new bulky alpha-substituents into these succinate-based hydroxamic acids was studied. Substituents such as thioethers, sulfonamides, and ethers showed improved potency against TACE when compared with Marimastat. Although this improvement did not translate into better blood potency for thioether or ether substituents, the sulfonamide series exhibited improved potency both against TACE and in blood when compared with Marimastat. Optimization of this sulfonamide series has culminated in the identification of heterocyclic bicyclic sulfonamides such as 3t (TACE IC(50): 0.57 nM; blood IC(50): 0.28 microM).

MeSH terms

  • ADAM Proteins
  • ADAM17 Protein
  • Administration, Oral
  • Animals
  • Callithrix
  • Humans
  • Hydroxamic Acids / chemical synthesis*
  • Hydroxamic Acids / chemistry
  • Hydroxamic Acids / pharmacokinetics
  • Hydroxamic Acids / pharmacology
  • Metalloendopeptidases / antagonists & inhibitors*
  • Metalloendopeptidases / blood
  • Protease Inhibitors / chemical synthesis*
  • Protease Inhibitors / chemistry
  • Protease Inhibitors / pharmacokinetics
  • Protease Inhibitors / pharmacology
  • Quinazolines / chemical synthesis*
  • Quinazolines / chemistry
  • Quinazolines / pharmacokinetics
  • Quinazolines / pharmacology
  • Succinates / chemical synthesis*
  • Succinates / chemistry
  • Succinates / pharmacokinetics
  • Succinates / pharmacology
  • Tumor Necrosis Factor-alpha / antagonists & inhibitors*
  • Tumor Necrosis Factor-alpha / metabolism

Substances

  • Hydroxamic Acids
  • N(2)-(4-(N-hydroxyamino)-2-isobutyl-3-(4-oxo-3,4-dihydroquinazoline-6-sulfonylamino)succinyl)-tert-leucine-N(1)-methylamide
  • Protease Inhibitors
  • Quinazolines
  • Succinates
  • Tumor Necrosis Factor-alpha
  • ADAM Proteins
  • Metalloendopeptidases
  • ADAM17 Protein
  • ADAM17 protein, human