Discovery of orally active hepatoselective glucokinase activators for treatment of Type II Diabetes Mellitus

Bioorg Med Chem Lett. 2017 May 1;27(9):2063-2068. doi: 10.1016/j.bmcl.2016.10.088. Epub 2016 Oct 31.

Abstract

Systemically acting glucokinase activators (GKA) have been demonstrated in clinical trials to effectively lower blood glucose in patients with type II diabetes. However, mechanism-based hypoglycemia is a major adverse effect that limits the therapeutic potential of these agents. We hypothesized that the predominant mechanism leading to hypoglycemia is GKA-induced excessive insulin secretion from pancreatic β-cells at (sub-)euglycemic levels. We further hypothesized that restricting GK activation to hepatocytes would maintain glucose-lowering efficacy while significantly reducing hypoglycemic risk. Here we report the discovery of a novel series of carboxylic acid substituted GKAs based on pyridine-2-carboxamide. These GKAs exhibit preferential distribution to the liver versus the pancreas in mice. SAR studies led to the identification of a potent and orally active hepatoselective GKA, compound 6. GKA 6 demonstrated robust glucose lowering efficacy in high fat diet-fed mice at doses ⩾10mpk, with ⩾70-fold liver:pancreas distribution, minimal effects on plasma insulin levels, and significantly reduced risk of hypoglycemia.

Keywords: Diabetes; Glucokinase; Glucokinase activator (GKA); Glucose homeostasis; Glucose metabolism; Hepatoselective; Hepatospecific; Hexokinase IV; Liver preferring; Pyridine-2-carboxamide; Type II Diabetes Mellitus.

MeSH terms

  • Animals
  • Diabetes Mellitus, Type 2 / blood
  • Diabetes Mellitus, Type 2 / drug therapy*
  • Diabetes Mellitus, Type 2 / metabolism
  • Drug Discovery
  • Enzyme Activators / chemistry
  • Enzyme Activators / pharmacokinetics
  • Enzyme Activators / pharmacology*
  • Enzyme Activators / therapeutic use
  • Glucokinase / metabolism*
  • Humans
  • Hypoglycemic Agents / chemistry
  • Hypoglycemic Agents / pharmacokinetics
  • Hypoglycemic Agents / pharmacology*
  • Hypoglycemic Agents / therapeutic use
  • Insulin / blood
  • Liver / drug effects
  • Liver / metabolism
  • Mice
  • Mice, Inbred C57BL
  • Pancreas / drug effects
  • Pancreas / metabolism
  • Pyridines / chemistry
  • Pyridines / pharmacokinetics
  • Pyridines / pharmacology*
  • Pyridines / therapeutic use

Substances

  • Enzyme Activators
  • Hypoglycemic Agents
  • Insulin
  • Pyridines
  • Glucokinase